We use Citibank for checking/large expense savings (we do everything online, I don't think they have a branch within 500 miles of here)
We use GMAC for e-savings / CD ladders. Good rates, great support. Workable website.
I use US Bank for a local branch. I keep my business checking account there and we have a personal checking account for standard transactions (notorize / medallion for free, deposit and transfer out, ATM, etc). Very helpful staff... but then, they have a branch office inside of BBY (where my wife works) so that probably influences things a lot.
Vanguard for the bulk of our assets (targeted retirement funds for IRA, index funds for taxable investing). I've been extremely pleased with the entire move and their customer service / support.
Fidelity for my wife's ESPP. Great site, decent customer support.
Schwab for individual stocks. Vanguard's brokerage account is a bit painful if you don't have enough assets with them.
It's a lot of accounts, but it's extremely transparent with MS Money / Quicken (used Money for 7 years, switched to Quicken and loving it). Citibank and GMAC are painless to pull money in and out online, no matter where your institution is.