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For carpenter ants, I used carbaryl dust (Sevin). In a hand dust pump, pump it directly on the ants, and any entry/exits they use. They pick up and carry the dust back to the nest and die there later, tracking and carrying a bunch of it along with them. Eventually the nest gets a critical mass of the dust and they either die off or decide to move the nest.
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Many an optimist has become rich by buying out a pessimist
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